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Beilstein J. Org. Chem. 2018, 14, 2698–2707, doi:10.3762/bjoc.14.247
Graphical Abstract
Scheme 1: ROM of various bicyclic unsaturated β-lactams [14-16].
Scheme 2: ROM of various constrained bicyclic unsaturated systems (γ-lactones, δ-lactones, γ-lactam, isoxazol...
Figure 1: Commercial Ru-based catalysts used in the current work.
Scheme 3: ROM of lactones (±)-3 and (±)-4.
Scheme 4: ROM of lactones (±)-9.
Scheme 5: ROM of structurally constrained bicyclic lactones and lactams.
Scheme 6: ROM of bridged lactone (±)-14 and cyclooctene-fused isoxazoline (±)-16.
Scheme 7: ROM and transformations of lactam (±)-18.
Figure 2: Chelate intermediates in CM of (±)-19.